Ok, first would be to sell off all your 2 stroke stuff to help fund your new motor swap project. Then figure out how many cc's you want/need for the class(s) you will race in. I'm limited to 140cc's so I went with the Tak 124cc kit and love it! If u want a cheap kit, BBR is a good one, or just a Tak 115 kit or Powroll 110 piston with inner-rotor kit and aftermarket cam... Yeah baby!!! To unleash all the power in these motors, you will need a super head with larger valves and ports, but they are not cheap!
Next you need a motor, then a bracket kit (wink, wink) to fit the XR/CRF100 motor in the NSR frame.
Then get the electrical/wiring harness for the 4 stroke (if it didn't come with the motor) It will be very straight forward to hook up. Also grab a extra long clutch cable and the clutch cable holder (it should come with the motor).
A stock carb will work, but if u can go with a bigger carb I would! The XR200 carb is a good cheap carb that people use with nice results! A different 24mm carb can be used as well depending on how crazy u go with your motor (I use a PE28mm carb). The intake can be made (see link below) or buy a offset NSF intake to point the carb straight back!
Cut off all tabs on the inside of your frame where all the 2 stroke electrical stuff was bolted to. This is the only stuff that needs cut
After u have the bracket kit (wink, wink), motor installed and electrical hooked up, you are almost done.
Next would be an exhaust. Either find a stock NSF exhaust or buy an aftermarket one from a guy with the initials BW in Texas. He has made some really good exhausts for both the NSR and NSF.
Or you can build your own exhaust, I've done that before and it worked great!
After all that, then it's time to have fun and enjoy the dark side!!! Mahahaha!!
More info on how I transformed my NSR50 into a NSF124 can be found here;
Brian's NSR-120RR
NSR50 to NSF-125cc
I say the CRF/XR swap is the best because it is all bold on, and no need for welding new mounts braces etc!! Plus, if u really wanted to go back to a 2 smoke, you can... The only thing u cut off are the small mounts for electrical stuff, that can be zip-tied on if swap'n back over.
Let me know if u have anymore questions... I love to help out others looking to swap over!!